《Microbial Electrochemical and Fuel Cells：Fundamentals and Applications》
《Microbial Electrochemical and Fuel Cells：Fundamentals and Applications》微生物燃料电池和电化学：基础和应用
编辑：Keith Scott and Eileen Hao Yu
出版社：WP
出版时间：2016年
目录
Contributors ix
Woodhead Publishing Series in Energy xi
Part One The workings of microbial fuel cells 1
1 An introduction to microbial fuel cells 3
K. Scott
1.1 Introduction 3
1.2 Fuel cells 4
1.3 Biological FCs 9
1.4 The MFC 11
1.5 Biological enzyme FC 24
1.6 Conclusions 25
References 26
2 Electrochemical principles and characterization of
bioelectrochemical systems 29
K. Scott
2.1 Introduction 29
2.2 Electrochemical principles 30
2.3 Voltammetric electrochemical methods 41
2.4 Rotating disk and ring-disk electrodes 49
2.5 Electrochemical impedance spectroscopy 52
2.6 Chronoamperometry 59
2.7 Square wave voltammetry 61
2.8 Differential pulse voltammetry 62
2.9 Other techniques 62
References 63
Further reading 66
3 Electron transfer mechanisms in biofilms 67
J. Philips, K. Verbeeck, K. Rabaey and J.B.A. Arends
3.1 Introduction 67
3.2 Mechanisms for delivering electrons to an anode 73
3.3 Mechanisms for electron uptake from cathodes 82
3.4 EET between microorganisms 92
3.5 Future trends and research needs 96
3.6 Conclusion 98
Acknowledgments 99
References 99
Further reading 113
Part Two Materials for microbial fuel cells and
reactor design 115
4 Anode materials for microbial fuel cells 117
A. Dumitru and K. Scott
4.1 Introduction 117
4.2 Anode materials 118
4.3 Surface modification of MFC anode materials 125
4.4 Conclusions and future perspective 144
References 146
Further reading 152
5 Membranes and separators for microbial fuel cells 153
K. Scott
5.1 Introduction 153
5.2 Cell separators 155
5.3 Transport processes in membranes and diaphragms 158
5.4 Membranes for microbial fuel cells 161
5.5 Future trends 175
References 176
Bibliography 177
6 Cathodes for microbial fuel cells 179
S. Bajracharya, A. ElMekawy, S. Srikanth and D. Pant
6.1 Introduction 179
6.2 Redox reactions for MFCs 179
6.3 The oxygen reduction mechanism 183
6.4 Hydrogen evolution mechanism 189
6.5 ORR cathode configuration in MFC 192
6.6 Non-precious metal cathodes 193
6.7 Enzymatic cathodes 198
6.8 Future trends 205
Acknowledgment 205
References 206
7 Reactor design and scale-up 215
G.C. Premier, I.S. Michie, H.C. Boghani, K.R. Fradler and J.R. Kim
7.1 Introduction 215
7.2 Performance indicators for MFCs 216
vi Contents
7.3 What governs the performance of MFCs 222
7.4 Determining the performance of MFCs 224
7.5 MFC architectures 228
7.6 Connectivity and control mechanisms 230
7.7 MFC scale-up, application, and integration 235
7.8 Future trends 237
References 239
Part Three Applications of microbial electrochemical
and fuel cells 245
8 Microbial fuel cells for wastewater treatment and energy
generation 247
V.G. Gude
8.1 Wastewater treatment 247
8.2 Wastewater–energy–environment nexus 247
8.3 Energy requirements for wastewater treatment 249
8.4 Energy recovery in wastewater treatment systems 251
8.5 Microbial fuel cells 254
8.6 Organic removal in MFCs 260
8.7 Algae biocathode for MFCs 266
8.8 Nitrogen removal in MFCs 268
8.9 Phosphorus removal in MFCs 271
8.10 Metals removal in MFCs 272
8.11 Source separation 274
8.12 Conclusions 275
Acknowledgments 276
References 276
9 Microbial electrolysis cells for hydrogen production 287
S. Cotterill, E. Heidrich and T. Curtis
9.1 Introduction 287
9.2 Advantages 289
9.3 Disadvantages 290
9.4 Role in the hydrogen economy 290
9.5 How to characterize an MEC 291
9.6 Rhetoric to reality? 295
9.7 Problems 312
9.8 Beyond hydrogen 314
9.9 Prospects for deployment of MEC 314
9.10 Conclusions: How to make MECs happen? 315
Further reading 316
References 316
Contents vii
10 Resource recovery with microbial electrochemical systems 321
E.H. Yu
10.1 Introduction 321
10.2 Metal recovery 322
10.3 Nutrients removal and recovery 328
10.4 Converting CO2 to valuable chemicals 332
10.5 Prospective 334
References 335
11 Use of microbial fuel cells in sensors 341
M. Di Lorenzo
11.1 An introduction to biosensors 341
11.2 Microbial biosensors 341
11.3 The use of microbial fuel cells as electrochemical sensor 342
11.4 Operation of the MFC sensor 343
11.5 MFC sensor design 346
11.6 MFCs as BOD sensors 347
11.7 Detection of toxicants in water by MFCs 351
11.8 Conclusions 353
References 353
12 The practical implementation of microbial fuel cell technology 357
I. Ieropoulos, J. Winfield, I. Gajda, A. Walter, G. Papaharalabos,
I.M. Jimenez, G. Pasternak, J. You, A. Tremouli, A. Stinchcombe,
S. Forbes and J. Greenman
12.1 Introduction 357
12.2 Direct use of microbial fuel cells 358
12.3 Implementing energy harvesting 363
12.4 Field trials 372
12.5 Conclusions 378
References 378
Index 381
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